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No 30
Introduction of the research of Dr.Akinori Ito and Dr.Kentaro Ishijima
We have got the ability beyond other animals by controlling ignition. We used fires to clear land for our living. Now, most of the biomass burning takes place in the tropical belt and is associated with human practices. Warming and earlier spring will increase wildfire activity in boreal and temperate forests. The biomass burning is one of the most significant sources of trace gases and aerosols on a global scale and influence an air quality and climate. I deliver the "hot" research topics at the joint IGAC/CACGP/WMO Symposium, September 2006, Cape Town, South Africa. (Akinori Ito)
Since the industrialization in the 19th century, atmospheric concentrations of greenhouse gases such as carbon dioxide (CO2), methane (CH4) and nitrous oxide (N2O) have much increased due to human activities. Therefore, possible bad impacts on global environment, such as global warming and following climate change are the recent concerns. N2O has 300 times global warming potential of that of CO2, and is related to depletion of ozone layer, so recently the N2O research is getting important. At FRCGC, I am trying to understand the global cycle of N2O and to quantify its sources, by numerical simulation using a global model. (Kentaro Ishijima)

No 29
We are happy to introduce Dr. Masanori Niwano, who has joined our program in October. During his graduate-school years, he revealed seasonal and interannual variations of the Lagrangian upward velocity in the tropical lower stratosphere by using water vapor and methane data from HALOE on board UARS satellite, and contributed to the understanding of the transport processes and dynamics in the lower stratosphere.
During the post-doctoral years in Kyoto University, he examined geographical distribution of cirrus clouds, aerosol, and upwelling in the tropical tropospause region. In FRCGC, he will engage in establishing the regional chemical weather forecast system for Kanto region and study the role of transport in the occurrence of photochemical oxidant.


No 28
The Acid Rain 2005 Conference was held on 12-17 June 2005 in Prague, Czech Republic, andbrought together more than 600 scientists from more than 40 countries. Three researchers,i.e., DrsBin Zhu, Pakpong Pochanart and Xiaoyuan Yan, and one sub-leader, Dr. Toshimasa Ohara, fromAtmospheric Composition Program, attended the conference. Acid Rain is a series conference takingplace every 5 years. The previous Acid Rain was held in Tsukuba Japan, and the next one will be heldin Beijing, 2010 and chaired by Dr. Zifa Wang, an alumnus of Atmospheric Composition Program.


The focus of these conferences has evolved over the years starting with focus on questions regarding the causes and effects of acidrain, to measures required to reduce the problems, to the degree and rate of recovery, and now to the complicating role of otherpollutants. And it was proposed that the next conference be named Acid Rain and Air Pollution.The Acid rain problem originated from Europe and North America in 1970s withextensive damage to fish and risk to forest. Now in these regions, emissions of sulphurand nitrogen has declined, acidification of soil and surface water has ceased in large areas,and ecosystems are beginning to recover. However, emissions are increasing rapidlyelsewhere, especially in regions such as China, Japan, and the Indian sub-continent arenow at risk for damage to human health and to freshwater and terrestrial ecosystems.Thus more research and policy response are needed in these regions.


No 27
Prabir Patra attended AGU Chapman Conference on The Science and Technology of Carbon Sequestration at San Diego, 16-20 January 2005. This meeting was different in some sense from the conventional ones. All presentations were directed towards the application of our understanding of carbon cycle science, either in verification or assessment of natural and deliberate carbon sinks. The issue of forced increase in natural carbon sinks, such as the ocean sediments or terrestrial biosphere, and deliberate sinks in the oil wells or earth's crust were discussed in details. The consensus is multiple methodologies have to be implemented to control atmospheric CO2 increase. Note that the carbon sequestration science and technology are being developed to mitigate CO2 increase in our atmosphere, and to comply with the commitments each countries have made under the Kyoto Protocol. Though there may be technologies available at hand to sequester carbon, but its longer-term repercussions are not known, such as how to inject CO2 in the ocean without affecting the marine life. The verification of carbon-credit claims by each country is another serious problem, where he thinks we can contribute through inverse and forward modeling of CO2.



No 26

Two scientists, Dr. Hitoshi Irie and Dr. Donald Lucas, have joined the Atmospheric Composition Research Program this year. Before this March, Dr. Hitoshi Irie was working at National Institute for Environmental Studies (NIES) to address the issue on the formation process of polar stratospheric clouds, which play a central role in the Arctic ozone depletion, by using satellite data (ADEOS/ILAS) and a cloud microphysics model.
From these experiences, Dr. Irie would like to analyze satellite data at FRCGC to investigate temporal/spatial variations of atmospheric composition and to contribute to solving global environment issues. Dr. Donald Lucas joined our program in May. Dr. Lucas was previously at MIT, where he used a variety of computer models to study the atmospheric chemistry of dimethylsulfide, an important biogenic sulfur compound. At the FRCGC, Dr. Lucas plans to incorporate a size-resolved description of aerosols into a global 3D chemistry-climate model, which he will then use to quantify the production and fate of secondary aerosols in the troposphere.



No 25

   A major goal of the Global Chemical Transport Modelling Group is to investigate and quantify the links between air quality and climate through the impacts of tropospheric ozone. Ozone is the third most important trace gas affecting climate, after CO2 and methane, and has been increasing much more quickly - by a factor of 3-4 over the past century. This change has been accompanied by increasing levels of 'smog' ozone near the Earth's surface, which affect human health and agricultural crop yields, and has been principally attributed to human activities. To address this goal, Dr. Oliver Wild participated in the NASA TRACE-P atmospheric measurement campaign over the Western Pacific in Spring 2001, and has recently provided detailed analyses of the production of ozone in the highly polluted air transported out of East Asia which was intercepted over the Western Pacific by measurement aircraft. While sunny, anticyclonic conditions were found to contribute substantially to the build-up of pollutant ozone over China, the impacts on climate were found to be larger under cloudy conditions when regional build-up was small. This unexpected result highlights the complex relationships, which exist between regional pollution and global climate, and demonstrates the additional insight that can be gained by combining high-resolution chemistry model studies with detailed measurements of tropospheric trace gases and aerosols.

No 24

One of the activities in Atmospheric Composition Data Analysis Group is to study the changes in ozone variabilities (seasonal as well as long-term) over three continents, i.e. Europe, North America and Asia, which would help in estimating the influences of regional pollution and intercontinental transport. Recent numerical simulations suggest that ozone level in the Far East Asia is determined by regional scale photochemical buildup superimposed to the "northern-hemispheric background" that is controlled by the precursor emissions in Europe, North America and Asia itself. In this regard, it becomes necessary to formulate a suitable and versatile technique to analyze observational data. The residence times and sectoral classifications based analysis of ozone data shows that ozone, which is produced within European boundary layer decreases sharply after the year 1990. This is consistent with the change in NOx emissions over Europe. However, almost no change in ozone abundance in European lower troposphere is due to intercontinental transport of precursors from U.S.A. Large contribution of Chinese outflow has been observed in the ozone abundances over Japan in late spring/summer in the boundary layer and lower troposphere. Significant contribution of European outflow is also observed over Japan throughout the year. These observational proofs of long-range transport have important implications on deciding the background ozone levels and air-quality standards over a particular continent.

No 23

Croplands have been identified as a very important source of atmospheric trace gases such as N2O (nitrogen monoxide), NO (nitric oxide), NH3 (ammonia), and CH4 (methane). Agriculture in East, Southeast and South Asia exhibits unique factors related to the generation of these gases. Although this region accounts for only 36% of the world's cropland area, it consumes more than half of the world's nitrogen fertilizers. Moreover, approximately 90% of the world's rice fields, a source of CH4, are located in this region. Therefore, emissions of N2O, NO, NH3 and CH4 from croplands in this region merit the close scrutiny of Xiaoyuan Yan in the Emission Inventory Sub-Group. By analyzing the relationships between emissions and fertilizer use, soil properties, water management and climate, and by drawing upon agricultural activity data, we have developed a fine emission inventory of N2O, NO, NH3 and CH4 from croplands for each country in this region. For China and India, the inventory was developed for each province or state. In addition, we are trying to predict future emissions of these gases by considering changes in land use and population as well as economic growth.

No 22

A task team for atmospheric composition observation has been founded within the atmospheric composition research program. The observational work, which is a part of Ministry of Education, Culture, Sports, Science and Technology (MEXT) Research Revolution 2002 project, will focus on two topics, the long-term observation of large-scale air pollution in East Asia and intensive observation of the atmospheric radical species. Here we would like to introduce the long-term observation. As a result of fast economic growth in East Asia, massive amounts of air pollution, including those having direct impact on global warming, natural environment change, agricultural production loss, and human health, are being released into the atmosphere and are predicted to continue increasing. The study of the long-term variation of such large-scale air pollution in this region and the process and mechanism controlling such variations are in urgent need. Starting from the end of this fiscal year, continuous monitoring of ozone and carbon monoxide will be carried out in the highly populated region of China. The observation of background conditions of these species in remote Siberia will also be made. The observation results would give us the new information that helps validate and improve the atmospheric chemical-transport modeling and strengthen the capability to predict the status of air pollution in the future.

No 21

Report by Drs. Prabir K. Patra and Shamil Maksyutov. In the Greenhouse Gases Modeling Group, we are aiming to estimate the regional fluxes of carbon dioxide (CO2) by using the information from atmospheric data and its variability. Since most of the present CO2 measurement stations are located to keep track of the long-term background changes, the inverse model estimates of surface fluxes are not well determined on the regional scale. Our attention is focused on improving present measurement network of CO2 optimally for better regional source distribution. Such study is also recommended to observe the changes occurring under the Kyoto Protocol for mitigating the anthropogenic component of greenhouse gas emission, while increasing the terrestrial CO2 uptake in biomass. The implementation of optimal network simulation is generally probabilistic and computer-time consuming at present. We have introduced "incremental" optimization technique to study the dearth in currently operating CO2 measurement network and propose possible extensions in order to estimate regional fluxes of CO2 with greater confidence using inverse models. We have identified that the continental South America, Africa and some parts of Asia require more CO2 observations. Since new algorithm is less computer-time demanding, fifteen transport models are utilized in the inverse model calculations. This helps reducing uncertainties in the optimal extensions due to the inaccuracies in model transport. These results are in use while selecting the new observation sites under the recently funded CO2 observation projects.

No 20

10th Symposium of the IAMAS/CACGP (Commission of Atmospheric Chemistry and Global Air Pollution) and 7th Scientific Conference of the International Global Atmospheric Chemistry Project (IGAC) were jointly held during 18th-25th September in Crete Island, Greece.

Program Director, Dr. Hajime Akimoto, and 10 other colleagues of ACRP joined the meeting and contributed their latest achievements. The meeting, as it is titled "Atmospheric Chemistry within the Earth System: From Regional Pollution to Global Change," covers a wide range of issues on the tropospheric compositions -greenhouse gases, oxidants, acidic substances, and aerosols -including their natural variability, anthropogenic impacts exerted, and their roles in the context of global change. One of the highlights in this meeting was a cluster of presentations on ongoing as well as completed regional field studies across the globe, in which well-instrumented aircraft/ships/ground-based stations are intensively coordinated according to their scientific objectives.

Atmospheric chemists in Japan have surely contributed a lot in such activities especially in Asia and the western Pacific region. Huge database collected in field studies has helped and will keep helping a lot for validating and refining chemical-transport models.

At the end of the Symposium, Dr. Anne Thompson of NASA/GSFC succeeded as the next CACGP chair from Dr. Akimoto who had been serving as the chair since 1998.

No 19

Program Director, H. Akimoto attended "Air Pollution as a Climate Forcing Workshop" held in Honolulu during Aril 29 and May 3, midst of Golden Week. The venue was East West Center located in the cam-pus of University of Hawaii. The workshop was co-sponsored by IPRC together with NASA, NOAA, EPA, etc., and IPRC staff members took care of more than 100 participants.

The workshop theme was a link between non-CO2 air pollutants such as methane, ozone and aerosol, and climate change. Wide range of topics including atmospheric chemistry, mitigation technology, and health effects were discussed.

Akimoto met all Japanese members of IPRC during a session interval as well as the IPRC Director, Dr. McCeary, at the reception. It was very good to have had a chance to get acquainted directly with IPRC with which we usually do not have close contact.

No 18

How the airborne pollutants produced over the Asian continent are entering the western Pacific region? To answer this question, NASDA, in co-operation with domestic and foreign researchers, conducted the aircraft observation,The Pacific Exploration of Asian Continental Emission phase-A (PEACE-A), from 6 to 23 January.

During that period, Dr. Masayuki Takigawa, a researcher of our program stayed at the base of operations in Kagoshima. He provided the chemical weather forecast, which contributed greatly to the route making of the airplane. The forecasting system, developed by Dr. Takigawa, incorporated the emission, dispersion, and photochemical processes of about 30 chemical species into atmospheric general circulation model (AGCM).

It can thus predict the global distribution of photochemical oxidants, sulfate aerosols, and their precursors for up to 4 days. The system predicted the atmospheric flow of pollutants accompanying the cold front passage, which agreed well with the observation.


No 17

A Russian scientist Dr. Leonid Yurganov, who expertises a remote sensing technique of atmospheric trace elements, has joined FRCGC since last October. During the past several years of his stay in US and Canada, he has been working for the data validation team for a satellite sensor MOPITT (Measurements Of Pollution In The Troposphere). Satellite remote sensing of tropospheric chemical species is one of the promising and growing subjects, and atmospheric chemists worldwide are gathering around this "cutting edge" field.

By MOPITT horizontal distributions of CO and CH4 in the troposphere have been successfully retrieved on a global scale, which reveal their emissions into the atmosphere as well as their long-range transport across the globe. Dr. Yurganov is also challenging a retrieval of other tropospheric pollutants including NO2. At FRCGC, he will collaborate with chemical-transport modelers to make inter-comparisons between model results and satellite data.

No 16

In June, the Workshop on Emissions of Chemical Species and Aerosols was held in Paris. Program Director Dr. Akimoto, Sub-leader Dr. Ohara, researcher Dr. Yan, and research staff Ms. Yamaji attended the workshop and the emission inventory subgroup gave its first presentation. Dr. David Streets was invited from Argonne National Laboratory in the U.S. for a seminar at our institute on September 3. In collaboration with Dr. Streets, the Atmospheric Composition Research Program aims to develop a high-resolution emission inventory for the Asian region. In July, seven members of the research program participated in the 8th Scientific Assembly of InternationalAssociation of Meteorology and Atmospheric Sciences (IAMAS) in Innsbruck. The seven participants included Program Director Dr. Akimoto and researchers Drs. Wild, Takigawa, Zhang, Pochanart, Kanaya, and Naja. Preparations in the research program are also under way for the Symposium on Atmospheric Composition Change: Toward the Integration of Observation and Modeling, which will be held on November 19 and 20 at the Yokohama Institute for Earth Sciences.